Imaging the time-dependent structure of a molecule as it undergoes dynamics

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Title Imaging the time-dependent structure of a molecule as it undergoes dynamics
Author Legare, F.; Lee, Kevin F.; Litvinyuk, Igor; Dooley, P. W.; Bandrauk, A. D.; Villeneuve, D. M.; Corkum, P. B.
Journal Name Physical Review A (Atomic, Molecular and Optical Physics)
Year Published 2005
Place of publication United States
Publisher American Physical Society
Abstract We image the dynamics of diatomic and triatomic molecules with sub-5 fs and sub-A resolution using laser Coulomb explosion imaging with 8 fs pulses. We obtain image information by measuring the vector momenta of all atomic ions produced by explosion of a single molecule. We image vibrating D{sub 2}{sup +} and of dissociating SO{sub 2}{sup 2+} and SO{sub 2}{sup 3+}. Images taken at 0 and 60 fs show that the dissociation of SO{sub 2}{sup 2+} produces an SO{sup +} rotational wave packet.
Peer Reviewed Yes
Published Yes
Alternative URI http://dx.doi.org/10.1103/PhysRevA.72.052717
Volume 72
Issue Number 5
Page from 052717-1
Page to 052517-4
ISSN 1050-2947
Date Accessioned 2010-08-09
Date Available 2011-07-05T10:09:59Z
Language en_AU
Research Centre Centre for Quantum Dynamics
Faculty Faculty of Science, Environment, Engineering and Technology
Subject Atomic and Molecular Physics
URI http://hdl.handle.net/10072/39402
Publication Type Journal Articles (Refereed Article)
Publication Type Code c1x

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